Ferromagnetic stability in Fe nanodot assemblies on Cu(111) induced by indirect coupling through the substrate.
نویسندگان
چکیده
We report collective ferromagnetic behavior with high Curie temperatures (T(c)) in Fe dot assemblies supported by the Cu(111) surface. Our ability to tune the average size and spacing of the individual dots allows us to conclude that enhanced magnetic anisotropy cannot account for this high-T(c) ferromagnetic order. Because our Monte Carlo simulations have ruled out the dipolar interaction as the dominant factor in this system, we attribute the origin of the ferromagnetic order to indirect exchange coupling via the Cu(111) substrate.
منابع مشابه
Tuning substrate-mediated magnetic interactions by external surface charging: Co and Fe impurities on Cu(111)
The substrate-mediated magnetic interactions between substitutional Co and Fe impurities at the Cu(111) surface have been theoretically investigated as a function of external surface charging. The modification of the interactions as a result of the metallic screening and charge rearrangements are determined self-consistently from first principles by using the Green’s-function Korringa-Kohn-Rost...
متن کاملGrowth, structure, and magnetism of fcc Fe ultrathin films on Cu„111... by pulsed laser deposition
Ultrathin Fe films on Cu~111! have been grown by pulsed-laser deposition ~PLD! whose instantaneous deposition rate is about six orders of magnitude larger than that of the conventional molecular-beam epitaxy based on thermal deposition ~TD!. Compared to the TD prepared Fe/Cu~111! films, the PLD films have a significantly improved layer-by-layer morphology and a substantially enhanced stability ...
متن کاملStructure and magnetic properties of two cyanide - bridged one - dimensional M – CuII ( M FeIII or FeII ) bimetallic assemblies from ferricyanide and CuN
Two bimetallic assemblies K[Cu(cyclam)][Fe(CN)6] 4H2O 1 and [Cu(L)][Cu(L )][Fe(CN)6] 6.5H2O 2 (cyclam = 1,4,8,11-tetraazacyclotetradecane; L = N,N -bis(2-pyridylmethylene)-1,3-propanediamine and L = N-2-pyridylmethylene-1,3-propanediamine) have been prepared from the reaction of [Fe(CN)6] 3 and the precursors [Cu(cyclam)] and [Cu(L)] , respectively, and their structure and magnetic properties s...
متن کاملInvestigation and Modification of the Magnetism of Epitaxial Fe Structures
In this thesis, the magnetic and structural properties of layered epitaxial film systems and clusters are presented. A main achievement is the investigation of the direct correlation between magnetism and structural or morphological details of ultrathin films. For this purpose, the film structure has been accessed directly by means of surface science methods. The effect of structural changes on...
متن کاملExchange interaction of strongly anisotropic tripodal erbium single-ion magnets with metallic surfaces.
We present a comprehensive study of Er(trensal) single-ion magnets deposited in ultrahigh vacuum onto metallic surfaces. X-ray photoelectron spectroscopy reveals that the molecular structure is preserved after sublimation, and that the molecules are physisorbed on Au(111) while they are chemisorbed on a Ni thin film on Cu(100) single-crystalline surfaces. X-ray magnetic circular dichroism (XMCD...
متن کاملذخیره در منابع من
با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید
برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید
ثبت ناماگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید
ورودعنوان ژورنال:
- Physical review letters
دوره 92 23 شماره
صفحات -
تاریخ انتشار 2004